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Hydrogenation Process Flowsheets & Simulations

Explore 3 validated, solved Hydrogenation simulation flowsheets in MaximaLabs — real components: benzene, h2, cyclohexane, nitrobenzene, hydrogen, aniline. Open any one directly in your browser.

Solved via: PENG-ROBINSON.

Benzene
Hydrogen
MIX
RXN
SEP
Split
Cyclohexane
Purge
Reference model (ChemSep)

Benzene hydrogenation → cyclohexane

Benzene + 3 H₂ → cyclohexane in a conversion reactor, then a high-pressure flash recovers liquid cyclohexane and recycles the excess hydrogen (with a purge). The classic ChemSep recycle example — exercises reaction + recycle convergence.

8 unit ops • PENG-ROBINSON

227 0

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NB FEED
H2 FEED
MIX
RX
Hpsep
H2 VENT
Vflash
Water OVHD
Aniline Product
Ludwigshafen, Germany

Aniline via nitrobenzene hydrogenation

Vapor-phase catalytic hydrogenation of nitrobenzene (C₆H₅NO₂ + 3H2 → C₆H₅NH₂ + 2H2O, highly exothermic) with excess hydrogen, a high-pressure flash recovering unreacted H₂ as a recycle vent, then a reduced-pressure flash stripping residual water from the crude aniline.

9 unit ops • PENG-ROBINSON

224 0

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Nitrobenzene
Hydrogen
Loopmix
RX
Loophx
SEP
Offgas
Takeoff
Crude Aniline
Looppump
Aniline plant, Ludwigshafen, Germany

Jet loop reactor: nitrobenzene to aniline

A circulating loop reactor of the kind BASF and Buss built for strongly exothermic three-phase hydrogenations — here nitrobenzene to aniline (C₆H₅NO₂ + 3 H₂ → C₆H₅NH₂ + 2 H₂O, -443 kJ/mol). Fresh nitrobenzene and hydrogen are injected into a large circulating liquid stream; the reactor itself runs adiabatic and the reaction heat is taken out by a heat exchanger in the EXTERNAL loop, which is the whole architectural point — the exchanger area is set independently of the reactor, and the circulation rate, not a cooling jacket, is what holds the temperature. A gas separator vents the excess hydrogen, 5% of the liquid is taken off as crude aniline, and the rest is pumped back. What it computes: a 19:1 recycle-to-product ratio holds the adiabatic reactor to 429.7 K in / 494.3 K out, a 64.6 K rise, with the loop cooler removing 4.66 MW; overall nitrobenzene conversion is 99.98% (99.70% per pass) and the crude leaves at 34.7% aniline / 64.9% water. Counting the vent as well as the crude, one aniline is made per two water, which is the stoichiometric mass-balance check on the whole loop — the crude by itself runs slightly water-lean because the vent carries water vapour off with the excess hydrogen. The acid test is what happens without the loop: the same feed in one adiabatic once-through reactor is already at 627 K by 30% conversion and runs off the top of the model's temperature range well before full conversion. That gap is the reason the architecture exists.

10 unit ops • PENG-ROBINSON

76 0

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