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Acetic acid Process Flowsheets & Simulations

Explore 4 validated, solved Acetic acid simulation flowsheets in MaximaLabs — real components: methanol, carbon_monoxide, acetic_acid, water, diisobutyl_ketone, ethane. Open any one directly in your browser.

Solved via: PENG-ROBINSON, NRTL, NRTL-ASSOCIATE.

MEOH FEED
CO FEED
MIX
RX
Flash
CO VENT
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dist
btms
Qc
Qr
COL
Methanol Recycle
Acetic ACID Product
Acetic acid plant, Texas City, Texas, USA

Acetic acid via methanol carbonylation (Cativa process)

Methanol carbonylated with CO to acetic acid over the iridium-based Cativa catalyst (BP Chemicals), which runs at higher selectivity and lower water content than the older Monsanto rhodium process. The homogeneous catalyst itself isn't a flowing component in this model — only the carbonylation stoichiometry and downstream light-ends recovery are represented. Unreacted CO is flashed off and a column strips residual methanol from the acetic acid product.

9 unit ops • PENG-ROBINSON

227 0

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FEED
Solvent
feed
dist
btms
Qc
Qr
ED
Water Product
feed
dist
btms
Qc
Qr
SR
Acetic ACID Product
Solvent Recovered
Terephthalic acid plant, Map Ta Phut, Thailand

Dilute acetic acid recovery by extractive distillation

Recovering acetic acid from a dilute aqueous stream (e.g. cellulose acetate or terephthalic acid plant wastewater) using diisobutyl ketone (DIBK) as an extractive entrainer. Because acetic acid and water form no azeotrope but have a relative volatility that flattens toward 1 as the mixture concentrates, straight distillation needs an impractically tall column and heavy reboil duty; the entrainer raises water's relative volatility so the extractive column takes water overhead in far fewer stages, and a second column then strips the entrainer from the acid bottoms for recycle. Modeled with NRTL, and the property method is the whole point here rather than a detail: an entrainer works by changing liquid non-ideality, and a cubic equation of state with van der Waals mixing has no term for it — no binary interaction parameter ships for acetic-acid/water or DIBK/water, so Peng-Robinson runs this flowsheet at kij = 0 and represents none of the effect the column depends on. It does not converge either. NRTL carries the DECHEMA-fitted acetic-acid/water binary and reaches the DIBK pairs through UNIFAC.

7 unit ops • NRTL

226 1

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FEED
feed
dist
btms
Qc
Qr
COL
Water
ACID
Terephthalic-acid / cellulose-acetate plant, Map Ta Phut, Thailand

Acetic acid recovery — NRTL with vapor-phase dimerization

Concentrating dilute aqueous acetic acid (30 mol%) by distillation, modeled with the NRTL activity package and chemical-theory vapor-phase association (acetic acid dimerizes, 2 A → A2, in the vapor). This is the physics a cubic equation of state gets wrong: the pinned NRTL acetic-acid/water binary (DECHEMA) plus the cited dimerization constants (Nagy et al., Molecules 2020) give the real bubble curve and latent heat, so the close-boiling acid/water pair actually separates and converges where Peng-Robinson does not.

4 unit ops • NRTL-ASSOCIATE

224 0

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Illustrative EDHOX process (Linde/Clariant catalyst technology)

Oxidative dehydrogenation of ethane to ethylene + acetic acid (EDHOX concept)

Linde's EDHOX technology co-produces ethylene AND acetic acid from ethane and oxygen in one catalytic step (a proprietary mixed-metal catalyst in a multi-tubular salt-cooled reactor), with combined ethylene+acetic-acid selectivity published above 93% and the CO₂ by-product of over-oxidation recovered pure (no nitrogen dilution, since the oxidant is pure O₂, not air). Modeled here as three chained fixed-conversion reactors on real, exactly mass-balanced reactions: the main dehydrogenation (C₂H₆ + 0.5 O₂ → C₂H₄ + H₂O), the acetic-acid co-production path (C₂H₆ + 1.5 O₂ → CH₃COOH + H₂O), and a minor full-oxidation loss path (C₂H₆ + 3.5 O₂ → 2 CO₂ + 3 H₂O) accounting for the un-selective balance — the same 'illustrative, not fitted' posture as the naphtha cracker's furnace, since Linde's catalyst kinetics are proprietary and not published. The per-reaction conversions here are tuned to reproduce the one real published number (>93% combined selectivity: this flowsheet computes ~96%), not an assumed per-pass ethane conversion, which Linde doesn't publish.

10 unit ops • PENG-ROBINSON

186 0

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